Japan Geoscience Union Meeting 2015

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Symbol A (Atmospheric and Hydrospheric Sciences) » A-AS Atmospheric Sciences, Meteorology & Atmospheric Environment

[A-AS21] Atmospheric Chemistry

Thu. May 28, 2015 9:00 AM - 10:45 AM 201B (2F)

Convener:*Yousuke Sawa(Oceanography and Geochemistry Research Department, Meteorological Research Institute), Nobuyuki Takegawa(Graduate School of Science and Engineering, Tokyo Metropolitan University), Yugo Kanaya(Research Institute for Global Change, Japan Agency for Marine-Earth Science and Technology), Kenshi Takahashi(Research Institute for Sustainable Humanosphere, Kyoto University), Hiroshi Tanimoto(National Institute for Environmental Studies), Chair:Kengo Sudo(Graduate School of Environmental Studies, Nagoya University)

9:00 AM - 9:15 AM

[AAS21-06] Atmospheric Processing of Combustion Aerosols as a Source of Soluble Iron to the Open Ocean

*Akinori ITO1 (1.Japan Agency for Marine-Earth Science and Technology)

Keywords:Global environmental change, Atmospheric deposition, Soluble iron, Biomass burning

Atmospheric processing of combustion aerosols may promote transformation of insoluble iron into soluble forms. Here, an explicit scheme for iron dissolution of combustion aerosols due to photochemical reactions with inorganic and organic acids in solution is implemented in an atmospheric chemistry transport model to estimate the atmospheric sources of bioavailable iron. The model results suggest that deposition of soluble iron from combustion sources contributes more than 40% of the total soluble iron deposition over significant portions of the open ocean in the Southern Hemisphere. A sensitivity simulation using half the iron dissolution rate for combustion aerosols results in relatively small decreases in soluble iron deposition in the ocean, compared with the large uncertainties associated with iron solubility at emission. More accurate quantification of the soluble iron burdens near the source regions and the open ocean is needed to improve the process-based understanding of the chemical modification of iron-containing minerals.