*Olivier Evrard1, Pierre Sabatier2, Pierre-Alexis Chaboche3,4, Thomas Chalaux Clergue1, Anthony Foucher1
(1.Laboratoire des Sciences du Climat et de l’Environnement (LSCE/IPSL), Université Paris-Saclay, UMR 8212 (CEA-CNRS-UVSQ), Gif-sur-Yvette, France, 2.EDYTEM, Université Savoie-Mont Blanc, CNRS, Le Bourget du Lac, France, 3.International Research Fellow of Japan Society for the Promotion of Science (Postdoctoral Fellowships for Research in Japan - Standard), Japan, 4.Institute of Environmental Radioactivity, Fukushima University, Japan)
Keywords:fallout radionuclides, sediment archives, Anthropocene, golden spike
Dating recent sediment archives (<150 years) constitutes a prerequisite for reconstructing soil erosion and deposition processes during the last several decades. Radiocesium (137Cs) emitted during thermonuclear bomb testing (~1950 - ~1980) and nuclear accidents (1986 and 2011) was generally used for identifying sediment sources or for establishing sediment core chronology based on discrete time markers. Although this method has been widely used during the last several decades, there is a lack of structured and comprehensive worldwide synthesis of both natural and artificial fallout radionuclides used for dating sediment cores in environmental and Earth sciences. The current literature overview was based on 573 articles published between 1977 and 2020, reporting the collection of 1351 individual sediment cores. This synthesis led to the identification of the worldwide distribution of discrete time markers associated with the thermonuclear bomb testing peak in 1963, the Chernobyl fallout, the Fukushima fallout, and the identification of 25 events induced by local accidents or nuclear tests (e.g., Sellafield, la Hague accidents, Chinese nuclear tests).
With a growing number of studies focusing on the analysis of recent sediment cores and the increasing interest in sediment fingerprinting techniques, this spatialized synthesis provides a unique worldwide for identifying the distribution of 137Cs sources across the globe. The potential associated with the analysis of other fallout radionuclides, including excess-lead-210 (210Pbxs) and plutonium atom ratios (240Pu/239Pu), is also discussed to improve the dating of environmental archives for reconstructing soil erosion and sedimentation processes.