2015年 第76回応用物理学会秋季学術講演会

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一般セッション(口頭講演)

10 スピントロニクス・マグネティクス » 10.3 GMR・TMR・磁気記録技術

[14p-2J-1~4] 10.3 GMR・TMR・磁気記録技術

2015年9月14日(月) 13:45 〜 14:45 2J (223)

座長:後藤 穣(阪大)

14:00 〜 14:15

[14p-2J-2] CPP-GMR devices using Co2Fe(Ga0.5Ge0.5) full Heusler alloy and a AgZn alloy spacer

〇(D)YE DU1,2, Takao Furubayashi1, Taisuke Sasaki1, Yuya Sakuraba1, Yukiko Takahashi1, Kazuhiro Hono1,2 (1.NIMS, 2.Univ. Tsukuba)

キーワード:CPP-GMR,Heusler alloy,Spintronics

The current-perpendicular-to-plane giant magnetoresistance (CPP-GMR) devices with a metallic spacer layer have been considered to be promising for read sensors of ultrahigh density hard disk drives (HDDs). Using a Ag spacer layer, the MR ratios have reached over 50% with the resistance-change area product (dRA) reaching 9-12 mohm um2. However, a room-temperature dRA of at least 15 mohm um2 is required to use CPP-GMR as a read sensor for the areal density of over 2 Tbit/in2. In this work, we report a very large MR output obtained from the CPP-GMR devices that use CFGG Heusler alloy as ferromagnetic layers combined with an Ag-Zn alloy spacer.
Fully epitaxial multi-layer stacks of Cr(10)/Ag(100)/CFGG(10) /AgZn(5)/CFGG(10)/Ag(5)/Ru(8) (thickness in nm) were deposited onto (001) MgO single-crystalline substrates at room temperature (RT) by ultrahigh vacuum magnetron sputtering with a base pressure lower than 4×10-7 Pa. The CFGG and AgZn layers were deposited from alloy targets. The compositions of the deposited films examined by the induced coupled plasma analysis were Co47.2Fe25.9Ga13.5Ge13.4 and Ag50.2Zn49.8 (at%). The top CFGG layer was annealed right after deposition with annealing temperature (Tan) ranging from 350degC to 630degC. The samples were fabricated into CPP-GMR devices using electron beam lithography and Ar milling. The area of the pillar was measured by scanning electron microscopy. The microstructure was characterized by transmission electron microscopy (TEM).
Intrinsic MR ratio of 25.6% with dRA of 10.9 mohm um2 was obtained in the sample annealed at 350degC and MR ratio of 59.6% with dRA of 21.5 mohm um2 in the sample annealed at 630degC (Fig. 1). The structure of AgZn was found to be B2 in the as-deposited state; however, it changes to fcc after annealing at 350degC. At 630degC, Zn diffuses out of the spacer region (Fig. 2). The diffusion of Zn at 630degC improves the degree of ordering in CFGG, thereby enhancing the MR output. This work shows that the CPP-GMR devices with the AgZn spacer layer are promising for readers for high-density HDDs. The method for obtaining high spin polarization by utilizing the diffusion of Zn would be useful not only for CPP-GMR but also for other spintronic applications.