*Michio Aoyama^1,2, Daisuke Sasano³, Yuichiro Kumamoto¹, Hiroshi Uchida¹ (1.Research Institue of Global Change, The Japan Agency for Marine-Earth Science and Technology (JAMSTEC) , 2.Center for Research in Isotopes and Environmental Dynamic, Faculty of Life and Environmental Sciences, University of Tsukuba, 3.Atmosphere and Ocean Department, Japan Meteorological Agency)